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A 2 to 4 °C warming episode, known as the Latest Maastrichtian warming event (LMWE), preceded the Cretaceous–Paleogene boundary (KPB) mass extinction at 66.05 ± 0.08 Ma and has been linked with the onset of voluminous Deccan Traps volcanism. Here, we use direct measurements of melt-inclusion CO₂concentrations and trace-element proxies for CO₂to test the hypothesis that early Deccan magmatism triggered this warming interval. We report CO₂concentrations from NanoSIMS and Raman spectroscopic analyses of melt-inclusion glass and vapor bubbles hosted in magnesian olivines from pre-KPB Deccan primitive basalts. Reconstructed melt-inclusion CO₂concentrations range up to 0.23 to 1.2 wt% CO₂for lavas from the Saurashtra Peninsula and the Thakurvadi Formation in the Western Ghats region. Trace-element proxies for CO₂concentration (Ba and Nb) yield estimates of initial melt concentrations of 0.4 to 1.3 wt% CO₂prior to degassing. Our data imply carbon saturation and degassing of Deccan magmas initiated at high pressures near the Moho or in the lower crust. Furthermore, we find that the earliest Deccan magmas were more CO₂rich, which we hypothesize facilitated more efficient flushing and outgassing from intrusive magmas. Based on carbon cycle modeling and estimates of preserved lava volumes for pre-KPB lavas, we find that volcanic CO₂outgassing alone remains insufficient to account for the magnitude of the observed latest Maastrichtian warming. However, accounting for intrusive outgassing can reconcile early carbon-rich Deccan Traps outgassing with observed changes in climate and atmospheric pCO₂. 

Late Cretaceous records of environmental change suggest that Deccan Traps (DT) volcanism contributed to the Cretaceous-Paleogene boundary (KPB) ecosystem crisis. However, testing this hypothesis requires identification of the KPB in the DT. We constrain the location of the KPB with high-precision argon-40/argon-39 data to be coincident with changes in the magmatic plumbing system. We also found that the DT did not erupt in three discrete large pulses and that >90% of DT volume erupted in <1 million years, with ~75% emplaced post-KPB. Late Cretaceous records of climate change coincide temporally with the eruption of the smallest DT phases, suggesting that either the release of climate-modifying gases is not directly related to eruptive volume or DT volcanism was not the source of Late Cretaceous climate change. 

Abstract Deccan Traps flood basalt volcanism affected ecosystems spanning the end‐Cretaceous mass extinction, with the most significant environmental effects hypothesized to be a consequence of the largest eruptions. The Rajahmundry Traps are the farthest exposures (~1,000 km) of Deccan basalt from the putative eruptive centers in the Western Ghats and hence represent some of the largest volume Deccan eruptions. Although the three subaerial Rajahmundry lava flows have been geochemically correlated to the Wai Subgroup of the Deccan Traps, poor precision associated with previous radioisotopic age constraints has prevented detailed comparison with potential climate effects. In this study, we use new⁴⁰Ar/³⁹Ar dates, paleomagnetic and volcanological analyses, and biostratigraphic constraints for the Rajahmundry lava flows to ascertain the timing and style of their emplacement. We find that the lower and middle flows (65.92 ± 0.25 and 65.67 ± 0.08 Ma, ±1σsystematic uncertainty) were erupted within magnetochron C29r and were a part of the Ambenali Formation of the Deccan Traps. By contrast, the uppermost flow (65.27 ± 0.08 Ma) was erupted in C29n as part of the Mahabaleshwar Formation. Given these age constraints, the Rajahmundry flows were not involved in the end‐Cretaceous extinction as previously hypothesized. To determine whether the emplacement of the Rajahmundry flows could have affected global climate, we estimated their eruptive CO₂release and corresponding climate change using scalings from the LOSCAR carbon cycle model. We find that the eruptive gas emissions of these flows were insufficient to directly cause multi‐degree warming; hence, a causal relationship with significant climate warming requires additional Earth system feedbacks.